OperaV1, Main, Exploration, bibRecord, 000018

Seamless growth of a supramolecular carpet.

Identifieur interne : 000018 ( Main/Exploration ); précédent : 000017; suivant : 000019

Seamless growth of a supramolecular carpet.

Auteurs : Ju-Hyung Kim [Japon] ; Jean-Charles Ribierre [Japon] ; Yu Seok Yang [Japon] ; Chihaya Adachi [Japon] ; Maki Kawai [Japon] ; Jaehoon Jung [Japon] ; Takanori Fukushima [Japon] ; Yousoo Kim [Japon]

Source :

Nature communications ; 2016.

RBID : pubmed:26839053

Abstract

Organic/metal interfaces play crucial roles in the formation of intermolecular networks on metal surfaces and the performance of organic devices. Although their purity and uniformity have profound effects on the operation of organic devices, the formation of organic thin films with high interfacial uniformity on metal surfaces has suffered from the intrinsic limitation of molecular ordering imposed by irregular surface structures. Here we demonstrate a supramolecular carpet with widely uniform interfacial structure and high adaptability on a metal surface via a one-step process. The high uniformity is achieved with well-balanced interfacial interactions and site-specific molecular rearrangements, even on a pre-annealed amorphous gold surface. Co-existing electronic structures show selective availability corresponding to the energy region and the local position of the system. These findings provide not only a deeper insight into organic thin films with high structural integrity, but also a new way to tailor interfacial geometric and electronic structures.

DOI: 10.1038/ncomms10653
PubMed: 26839053

Affiliations:

Japon

Le document en format XML

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<front><div type="abstract" xml:lang="en">Organic/metal interfaces play crucial roles in the formation of intermolecular networks on metal surfaces and the performance of organic devices. Although their purity and uniformity have profound effects on the operation of organic devices, the formation of organic thin films with high interfacial uniformity on metal surfaces has suffered from the intrinsic limitation of molecular ordering imposed by irregular surface structures. Here we demonstrate a supramolecular carpet with widely uniform interfacial structure and high adaptability on a metal surface via a one-step process. The high uniformity is achieved with well-balanced interfacial interactions and site-specific molecular rearrangements, even on a pre-annealed amorphous gold surface. Co-existing electronic structures show selective availability corresponding to the energy region and the local position of the system. These findings provide not only a deeper insight into organic thin films with high structural integrity, but also a new way to tailor interfacial geometric and electronic structures.</div>
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Seamless growth of a supramolecular carpet.

Seamless growth of a supramolecular carpet.

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